Ultrafast Relaxation Dynamics of Uracil Probed via Strong Field Dissociative Ionization
We study the ultrafast relaxation dynamics of uracil excited to the first bright pi pi* state (S-2) by an ultrafast laser pulse in the deep ultraviolet (central wavelength lambda(0) = 260 nm). With a unique combination of strong field dissociative ionization measurements, state of the art strong field ionization calculations, and high level ab initio calculations of excited neutral and ionic state
